Preheat the oven to 375°F. Grease a skillet with 1 teaspoon unsalted butter (at room temperature).
Place 5 cups frozen unsweetened mixed berries in the greased skillet. Drizzle 1 tablespoon freshly squeezed lemon juice over the berries and spread them into an even layer.
In a small bowl, whisk together 2/3 cup granulated white sugar and 2 tablespoons cornstarch until combined. Sprinkle this mixture evenly over the berries and gently stir once or twice to coat.
In a medium bowl, combine 1 cup all-purpose flour, 2/3 cup packed dark brown sugar, 1 teaspoon ground cinnamon, and 1/4 teaspoon salt; mix to combine.
Add 1/2 cup (1 stick) cold unsalted butter, cubed, to the flour mixture. Using a pastry blender, two knives, or your fingertips, cut the butter into the dry ingredients until pea-sized pieces remain. Then use your fingertips to press and pinch the mixture into larger clumps to form the crumble topping.
Sprinkle the crumble topping evenly over the berry layer, covering as much of the berries as possible.
Bake in the preheated oven for 45 to 60 minutes, or until the topping is golden brown and the fruit filling is bubbling.
Remove the skillet from the oven and place it on a wire rack. Let the crumble cool for 15 minutes.
Spoon the crumble into individual serving bowls and top with vanilla ice cream, if using.